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Effect of gamma irradiation on the Ac-Dielectric properties of GaSe single crystals

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The Fifth Conference “ Nuclear Science and Its Application”, 14-17 October 2008

EFFECT OF GAMMA IRRADIATION ON THE AC-DIELECTRIC

PROPERTIES OF GASE SINGLE CRYSTALS

S.N. MUSTAFAEVA. A.A. ISMAILOV

Institute of Physics, National Academy of Sciences of Azerbaijan, Baku E-mail: [email protected]

GaSe crystals are layered wide-gap semiconductors with a rather high dc resistivity at 300 K. The purpose o f this work was to investigate the ac-dielectric properties o f GaSe single crystals and influence o f gamma irradiation on dielectric coefficients o f studied crystals.

The single-crystal GaSe samples for dielectric measurements had the form of planar capacitors normal to the C axis of the crystal, with silver-paster electrodes. The thickness o f the GaSe samples was 200pm. The dielectric properties of the GaSe single crystals were studied by a resonance technique using a TESLA BM 560 Q-meter. Loss tangent (tan8), real (e) and imaginary (e") parts of complex dielectric permittivity o f GaSe have been studied in the frequency range f = 5-104 to 3.5T07 Hz. All the measurements were performed at 300 K in alternate electric fields Section IV. Application O f Nuclear Technologies In Industry, Medicine And Agriculture

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The Fifth Conference “ Nuclear Science and Its Application”, 14-17 October 2008

corresponding to Ohmic current-voltage behavior. Co60 serves as the source of irradiation with energy of y-quantum equal to 1.3 MeV. The dielectric coefficients of non-irradiated and y-irradiated GaSe crystals were measured under the same conditions. As a result of the measurements conducted, it has been revealed that in the case o f the high frequencies (£>2-105 Hz) of the alternate electric field applied to the crystal the dielectric permittivity o f the specimen showed no significant variation due to y-irradiation, whereas in the case of the frequencies f<2T05 Hz, the s value decreased by two times as a result o f irradiation. For example prior to y-irradiation the e value at f=5T04 H z amounts to 8.3, whereas after irradiation (with dose 50kR) this value amounts to 4.1. At f=5 104 Hz the imaginary (s") part of complex dielectric permittivity of GaSe almost doubled as a result of y-irradiation.

Increasing the frequency from 5T04 to 3.5T07 Hz reduces the s of GaSe by more than a factor of 5 and that of y-irradiated GaSe by a factor of 2.7. The observed monotonic reduction in the dielectric permittivity of non-irradiated and y-irradiated GaSe single crystals with increasing frequency attests to the relaxation nature of the dispersion. The frequency dependences of the loss tangent for the GaSe prior and after y-irradiation have maxima, which also point to relaxation losses.

Thus the y-irradiation leads to the modification of dispersion curves e(f), s"(f) and tan8(f) of GaSe single crystals. The operation by the dielectric coefficients of the studied GaSe single crystals due to y-irradiation gives perspective for the use of these objects as active materials for creating of various transducers and gamma detectors.

Section IV. Application O f Nuclear Technologies In Industry, Medicine And Agriculture

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